Zintl phase EuIn₂As₂ has garnered growing attention as an axion insulator candidate, triggered by the identification of a commensurate double-Q broken-helix state in previous studies, however, its periodicity and symmetry remain subjects of debate. Here, we perform resonant x-ray scattering experiments on EuIn₂As₂, revealing an incommensurate nature of the broken-helix state, where both the wave number and the amplitude of the helical modulation exhibit systematic sample dependence. Furthermore, the application of an in-plane magnetic field brings about a broken-fanlike state preserving the double-Q nature, which could be attributed to multiple-spin interactions in momentum space. We propose that the itinerant character of EuIn₂As₂, possibly induced by Eu deficiency, gives rise to the helical modulation and impedes the realization of a theoretically-predicted axion state with the collinear antiferromagnetic order.
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Gen et al. (2024) studied this question.
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