Orbital-selective correlations and renormalized electronic structure in LiFeAs

Multiorbital physics is important to both the correlation physics and topological behavior of quantum materials. LiFeAs is a prototype iron pnictide suitable for in-depth investigation of this issue. Its electronic structure is strikingly different from the prediction of the noninteracting description. Here, a multiorbital Hubbard model is studied using a U (1) slave-spin theory. We demonstrate a mechanism for a substantial change to the Fermi surface, namely, orbital selectivity of the energy-level renormalization cooperating with its counterpart in quasiparticle spectral weight. Using this effect, we show how the dominating features of the electronic structure in LiFeAs are understood by the local correlations alone. Our results set the stage to understand the origins and nature of both the unconventional superconductivity and likely electronic topology in this prototype iron pnictide and, more generally, reveal a remarkable degree of universality out of the seemingly complex multiorbital building blocks across a broad range of strongly correlated superconductors.