Observation of Surface State Suppression in Magnetic Weyl Semimetal NdAlSi

Understanding and mastering the control of surface states in topological materials are crucial steps for the development of future electronic devices and technologies that leverage the unique properties of these materials. Here, using angle-resolved photoemission spectroscopy, we provide a good case study of this by visualizing the electronic structure of a magnetic Weyl semimetal on both flat and uneven surfaces. Our observations reveal that the preparation of an uneven sample surface can effectively suppress all surface states in the Weyl semimetal NdAlSi, including topological surface Fermi arcs. This results in the observation of pure bulk states devoid of any Fermi energy shift. This discovery not only opens up a new avenue to directly study the pure bulk states of a Weyl semimetal using low photon energies in ARPES but also provides key insights into the control of the surface states in topological materials.