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November 21, 2025Nature CommunicationsOpen Access

Operando microimaging of crystal structure and orientation in all components of all-solid-state-batteries

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Authors

QJQuentin JacquetJCJacopo Cele'LCLara Casiez

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Overview

Operando imaging shows how crystal structure influences reaction mechanisms in solid-state batteries, highlighting conductivity issues during manufacturing.

Key Points

  • Delithiation limited by Li-rich insulating interface in dense electrodes, suggesting performance constraints.
  • X-ray micro-diffraction identified the crystalline nature of LiCoO2 under real-time condition—critical for application.
  • Operando study of all-solid-state batteries utilized multiple materials including LiCoO2 and Li metal—new insights into structure.
  • Supports the need for effective characterization methods to bridge understanding in battery component interactions during operation.

Cite This Study

Jacquet et al. (2025) studied this question.

synapsesocial.com/papers/6924e3f8c0ce034ddc34f334https://doi.org/10.1038/s41467-025-66306-6
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