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December 12, 2025ACS Applied Materials & Interfaces5 citations

Mitochondrial-Targeting Drug-Loaded Nanoparticles Reprogram Macrophage Metabolism via ROS/NO Co-elimination for Diabetic Wound Healing

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XZXuan ZhouZHZhidan HuangHYHuake Yang

Key Points

  • To investigate how mitochondrial-targeting nanoparticles can reprogram macrophage metabolism for improved healing in diabetic wounds.
  • Developed TPP-modified mitochondria-targeting nanoparticles with encapsulated aminooxyacetic acid and H-MnO2.
  • Assessed the effects of these nanoparticles on macrophage metabolism and inflammation in vitro.
  • Evaluated the effectiveness of nanoparticles in diabetic murine wound models for promoting healing.
  • Nanoparticles reduced levels of nitric oxide and reactive oxygen species in macrophages.
  • Shifted macrophage metabolism from aerobic glycolysis to oxidative phosphorylation.
  • Enhanced re-epithelialization and collagen deposition in diabetic wound models.

Abstract

Diabetic wounds pose a growing healthcare challenge, characterized by heavy M1 macrophage infiltration, reactive oxygen species (ROS) overproduction, tissue hypoxia, and cytokine storms. The diabetic microenvironment fails to support the critical M1-to-M2 macrophage phenotypic switch, trapping tissues in persistent pathological inflammation that disrupts natural healing processes. In this study, we developed triphenylphosphonium (TPP)-modified mitochondria-targeting nanoparticles, where liposomes encapsulated two metabolomically guided agents: aminooxyacetic acid (AOAA) to suppress nitric oxide (NO) production and hollow mesoporous manganese dioxide (H-MnO2) to scavenge mitochondrial ROS and supply O2. In vitro, after successful mitochondrial internalization by macrophages, the nanoparticles reduced NO and ROS levels, enhanced mitochondrial respiration, and reprogrammed macrophage metabolism─shifting from aerobic glycolysis to oxidative phosphorylation (OXPHOS). This metabolic shift drove macrophage transition from pro-inflammatory M1 to anti-inflammatory M2 and thus resolved aberrant inflammation. In diabetic murine wound models, TPP-L@H-MnO2@AOAA further validated its efficacy. By modulating macrophage repolarization, it promoted re-epithelialization and collagen deposition. Overall, these anti-inflammatory nanoparticles with sustained-release capability provide a promising therapeutic tool for clinical management of diabetic wounds.

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Cite This Study

Zhou et al. (2025) studied this question.

synapsesocial.com/papers/694019032d562116f28f6102https://doi.org/10.1021/acsami.5c19664
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