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February 2, 2026The Journal of Organic Chemistry2 citations

Visible-Light-Driven Copper Catalysis: A Green and Sustainable Approach to Chlorohydroxylation of Chalcones

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QSQi ShiSouthwest UniversityDLDong-Xiang LiSouthwest UniversityXWXing-Lan WangSouthwest University

Key Points

  • This research aims to develop a green method for converting chalcones into chlorohydrins using visible light and copper catalysis.
  • Used visible-light-induced copper catalysis at room temperature
  • Converted chalcone derivatives with varying substituents
  • Conducted preliminary mechanistic studies on chlorine radical generation
  • Successfully transformed chalcones into corresponding chlorohydrins
  • Showed efficiency with both electron-withdrawing and electron-donating groups
  • Indicated chlorine radicals play a role in the reaction mechanism

Abstract

This work reports a green and sustainable method of chlorohydroxylation of chalcone derivatives via visible-light-induced copper catalysis under room temperature conditions to chemoselectively convert chalcones into the corresponding chlorohydrins. This approach enables the efficient conversion of various chalcone derivatives with electron-withdrawing and electron-donating groups. Preliminary mechanistic studies indicated that chlorine radical (Cl·) generated through the ligand-to-metal charge transfer process can promote the efficient construction of chlorohydrin structures.

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Cite This Study

Shi et al. (2026) studied this question.

synapsesocial.com/papers/6980ff49c1c9540dea812286https://doi.org/10.1021/acs.joc.5c02788
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