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March 3, 20260 citationsOpen Access

Persistent incommensurate charge density wave in chalcogen-disordered 1T-TaSeTe

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JSJyoti SharmaSCSambit ChoudhuryMHMeng-Jie HuangDeutsches Elektronen-Synchrotron DESY

Key Points

  • The incommensurate charge density wave remains stable at low temperatures, indicating resilience despite chalcogen disorder.
  • Electrical resistivity behavior suggests a semiconductor-like nature due to the gapping of the Fermi surface by the charge density wave.
  • Bulk and surface-sensitive techniques were used to investigate the electronic properties of the mixed-chalcogen compound.
  • Results indicate that chalcogen substitution can preserve the emergent electronic features of this transition metal dichalcogenide.

Abstract

Charge density waves (CDWs) are a canonical interaction-driven electronic phenomenon with potential technological applications, such as collective electronic switching and local information storage. Here, we investigate the properties of the CDW in the mixed-chalcogen compound 1T-TaSeTe using bulk- and surface-sensitive diffraction and spectroscopy techniques and transport measurements. Compared to the pristine parent compound 1T-TaSe2, we find that the incommensurate CDW appears to remain incommensurate down to low temperatures. The CDW-induced gapping of the Fermi surface is pronounced and may explain the observed semiconductor-like electrical resistivity behavior in combination with chalcogen disorder. Our results demonstrate that disordered chalcogen substitution doping can modify, yet preserve, the characteristic emergent electronic properties of a transition metal dichalcogenide.

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Cite This Study

Sharma et al. (2025) studied this question.

synapsesocial.com/papers/69a75ad3c6e9836116a21292https://doi.org/10.3204/pubdb-2026-00366
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