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March 3, 2026Journal of the American Chemical Society3 citations

Dynamic Crystal Photonics: Mechanically Mobile Organic Nonlinear Optical Microring Resonators

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MCMelchi ChosenyahRSRajaram SwarajVNVladimir Novikov

Key Points

  • Dynamic control demonstrates significant photonic behavior in nonlinear optical microring resonators—showing robustness and versatility.
  • The microring resonators exhibit nonlinear optical emissions with frequency comb-type whispering-gallery modes for enhanced functionality.
  • Utilizing a cantilever tip, these resonators are mechanically reconfigurable, enabling 3D spatial control of their orientation and behavior.
  • May enable advanced applications in mechanophotonic systems through improved photonic trait retention during dynamic manipulations.

Abstract

This work investigates the photonic aspects of organic crystal microring resonators (MRRs) under mechanically driven multifaceted motions, thereby pioneering the concept of dynamic crystal photonics. The MRRs are fabricated via surface-tension-assisted self-assembly of 6,6'-((1E,1'E)-hydrazine-1,2-diylidenebis(methaneylylidene))bis(2,4-dibromophenol) (HDBP), exhibiting nonlinear optical (NLO) emission and frequency comb-type whispering-gallery modes. Interestingly, the MRRs are micromechanically reconfigurable into various strained architectures, including lifting, transferring, vertical standing, axial spinning, and wheel-like rolling, using an atomic force microscopy cantilever tip. The MRRs retained their photonic traits throughout these dynamic motions, underscoring their mechanical robustness. Notably, the demonstration of axial spinning and rolling locomotion extends the manipulation capabilities beyond 2D control, enabling complete 3D spatial control. These results lay the groundwork for next-generation mechanophotonic crystal systems, enabling precise, dynamic control of the spatial orientation and photonic behavior of soft organic elements.

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Cite This Study

Chosenyah et al. (2026) studied this question.

synapsesocial.com/papers/69a75cd8c6e9836116a260echttps://doi.org/10.1021/jacs.5c17711
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