Indirect electrochemical synthesis demonstrates new applications of imine-bonded covalent organic framework films, suggesting innovative materials for various uses.
We introduce an indirect electrochemical synthesis approach for imine-bonded COF films, using electrogenerated acid as a catalyst. A simple and tunable electrolysis system yields COF or its intermediate film under ambient conditions within minutes, and is broadly applicable across versatile monomers. Several applications based on the higher-order structures are also demonstrated.
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Sato et al. (2026) studied this question.
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