This research demonstrates improved ammonia production in lithium-mediated nitrogen reduction with fluoride additives, suggesting more efficient techniques for nitrogen conversion.
Nitrogen Reduction Reaction Adding F-additives with low lowest occupied molecular orbital energy during the electrochemical Li-mediated N2 reduction reaction results in the formation of LiF solid electrolyte interphases. This process effectively reduces the energy barrier for the hydrogenation of Li3N on the surface, thereby enhancing the efficient production of NH3. More in article number 2404525, Hyeyoung Shin, Yun Jeong Hwang, and co-workers.
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Shin et al. (2024) studied this question.
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