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March 21, 2026Journal of Agricultural and Food Chemistry2 citations

Application of Natural Sesquiterpene Lactone for Pesticide Discovery: Design, Synthesis, and Insecticidal Evaluation of Xanthatin Derivatives Featuring Isoxazoline, Arylvinyl, and Sulfone Motifs

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CYChun YangMHMingtao HeZZZhenzhen Zheng

Key Points

  • The study aims to develop and evaluate the insecticidal properties of xanthatin derivatives for pest control.
  • Developed derivatives of xanthatin featuring isoxazoline, arylvinyl, and sulfone motifs.
  • Conducted bioassays to assess insecticidal activity against larvae of Mythimna separata and Plutella xylostella.
  • Performed greenhouse trials to evaluate efficacy and mortality rates.
  • Utilized enzyme assays and molecular docking to identify primary targets like acetylcholinesterase.
  • Compounds IIa, IId, IIh, and IIIa exhibited 3.9-4.5-fold greater insecticidal efficacy than xanthatin.
  • Compound IIh achieved 81.7% corrected mortality and 79.9% leaf protection in greenhouse trials.
  • Derivatives showed significant oral toxicity against larvae of Plutella xylostella.
  • The compounds indicated reduced cytotoxicity toward human keratinocyte cells compared to xanthatin.

Abstract

Xanthatin, a natural sesquiterpene lactone, served as an agrochemical scaffold to develop three series of derivatives bearing isoxazoline, arylvinyl, and sulfone motifs in this work. Bioassays identified compounds IIa, IId, IIh, and IIIa as highly potent against prethird-instar larvae of Mythimna separata, exhibiting 3.9-4.5-fold greater insecticidal efficacy than xanthatin and inducing typical neurotoxic symptoms. In greenhouse trials, compound IIh (500 mg/L for 72 h) achieved 81.7% corrected mortality and 79.9% leaf protection against M. separata, highlighting its practical potential. These derivatives also showed significant oral toxicity against prethird-instar larvae of Plutella xylostella. Notably, they exhibited Reduced cytotoxicity toward the human keratinocyte cell line (HaCaT) relative to xanthatin indicated enhanced dermal safety profile. Combined enzyme assays and molecular docking identified acetylcholinesterase (AChE) as the primary target. These novel xanthatin-derived compounds offer high insecticidal potency and favorable safety profile, representing promising agrochemical candidates.

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Cite This Study

Yang et al. (2026) studied this question.

synapsesocial.com/papers/69be34886e48c4981c672afahttps://doi.org/10.1021/acs.jafc.5c16234
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