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April 1, 2026Journal of Materials Chemistry A0 citations

Decoding Mixed-Ion Effects in Halide Electrolytes: Entropy as a Unified Measure of Soft and Disordered Lattice

RCRenyu CaiShanghai Jiao Tong UniversityYYYang YuSouthwest Jiaotong UniversityHZHong ZhuShanghai Jiao Tong University

Key Points

  • This research aims to understand how ion mixing influences the ionic conductivity of halide electrolytes through lattice dynamics.
  • Analyzed the effects of ion mixing on halide solid-state electrolytes
  • Examined lattice dynamics and related entropy measures in various compositions
  • Conducted experiments to assess changes in ionic conductivity
  • Demonstrated that ion mixing significantly improves ionic conductivity
  • Found that entropy serves as a unified measure for both soft and disordered lattices
  • Noted specific changes in lattice structure correlated with improved performance

Abstract

Ion mixing has emerged as an effective strategy to modulate the ionic conductivity of halide-based solid-state electrolytes, yet the underlying mechanisms—particularly those involving lattice dynamics—remain elusive. Li lattice softening, manifested...

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Cite This Study

Cai et al. (2026) studied this question.

synapsesocial.com/papers/69cd7b475652765b073a9368https://doi.org/10.1039/d6ta00983b
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