A chemical protocol to design robust hybrid [Fe(Htrz)₂(trz)](BF₄)@SiO₂ nanoparticles (NPs) with sizes as small as 28 nm and ultrathin silica shells below 3 nm has been developed. These NPs present a characteristic abrupt spin transition with a subsequent decrease in the width of the thermal hysteresis upon reducing the NP size.
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Torres‐Cavanillas et al. (2019) studied this question.
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