Intense white laser of high spectral flatness via optical-damage-free water–lithium niobate module

A supercontinuum white laser with ultrabroad bandwidth, intense pulse energy, and high spectral flatness can be accomplished via synergic action of third-order nonlinearity (3rd-NL) and second-order nonlinearity. In this work, we employ an intense Ti:sapphire femtosecond laser with a pulse duration of 50 fs and pulse energy up to 4 mJ to ignite the supercontinuum white laser. Remarkably, we use water instead of the usual solid materials as the 3rd-NL medium exhibiting both strong self-phase modulation and stimulated Raman scattering effect to create a supercontinuum laser with significantly broadened bandwidth and avoid laser damage and destruction. Then the supercontinuum laser is injected into a water-embedded chirped periodically poled lithium niobate crystal that enables broadband and high-efficiency second-harmonic generation. The output white laser has a 10 dB bandwidth encompassing 413 to 907 nm, more than one octave, and a pulse energy of 0.6 mJ. This methodology would open up an efficient route to creating a long-lived, high-stability, and inexpensive white laser with intense pulse energy, high spectral flatness, and ultrabroad bandwidth for application to various areas of basic science and high technology.