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April 24, 2026The Journal of Physical Chemistry Letters2 citations

The Properties of Current Induced Chiral Phonons Recapitulate the Characteristics of the CISS Effect

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HNHanggai NuominFSFeng-Feng SongPZP Zhang

Key Points

  • The research aims to explore the role of chiral phonons in producing spin polarization associated with the CISS effect.
  • Employed a tight-binding helical model to analyze phonon angular momentum.
  • Investigated the Berry potential in a corrected Born-Oppenheimer Hamiltonian.
  • Examined the influence of electric current flow on phonon symmetry properties.
  • Showed that chiral phonons generated by electric currents reflect the symmetry characteristics of the CISS effect.
  • Found that reversing current flow or chirality in structures affects phonon angular momentum similarly to the CISS effect.
  • Indicated that chiral phonons could contribute to the CISS effect in current-carrying systems.

Abstract

Chiral phonons, with their intrinsic angular momentum, are potential contributors to the chiral induced spin selectivity (CISS) effect, which can induce significant spin polarization in the absence of strong spin-orbit coupling. An open question is how nonzero total phonon angular momentum may be generated. If chiral phonons are to underpin the observed CISS effect, they must have the symmetries observed in CISS experiments. That is, reversing the chirality or reversing the direction of the current flow through the active CISS structure should influence the phonon angular momentum in the same way that these sign reversals influence the CISS effect (i.e., reversing the current or inverting the structural chirality reverses the spin polarization). We use a tight-binding helical model to show how phonon angular momentum is generated from directional electric current flow and show that the phonons thus generated have the same symmetry properties as the CISS effect. We analyze the Berry potential of a nonadiabatically corrected Born-Oppenheimer Hamiltonian; the Berry potential originates in the current-carrying electronic states and acts as a pseudo vector potential that circularly polarizes phonons. We find that the chiral phonons produced by electrical currents have the symmetry characteristics of the CISS effect, suggesting that current-induced chiral phonons may plausibly provide a source that contributes to the CISS effect.

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Cite This Study

Nuomin et al. (2026) studied this question.

synapsesocial.com/papers/69eb0a66553a5433e34b4815https://doi.org/10.1021/acs.jpclett.6c00793
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