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April 30, 2026ACS Nano3 citations

Chemotherapeutic Agent-Loaded Nanoparticles Synergizing with X-ray Irradiation to Regulate Fibroblast-like Synoviocytes for Rheumatoid Arthritis Treatment

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ZHZhixin HanYFYiming FengYZYuxuan Zhang

Key Points

  • This research aims to develop an effective drug delivery system targeting inflamed joints in rheumatoid arthritis.
  • Constructed a nanosystem using gold nanoparticles, FAPI, and β-CD for targeted drug delivery.
  • Used collagen-induced arthritis mice to evaluate the therapeutic efficacy of the nanosystem combined with low-dose radiotherapy.
  • Employed single-cell profiling to analyze the effects on inflammation and fibroblast activation.
  • Significantly reduced inflammation by eliminating activated B cells (p<0.01).
  • Effectively suppressed the migration of fibroblast-like synoviocytes (p<0.05).
  • Achieved comprehensive transcriptome standardization after treatment with combination therapy.

Abstract

Rheumatoid arthritis (RA) is a chronic, systemic autoimmune disorder characterized by progressive joint destruction and erosive pathology. Synovitis is considered the hallmark pathological manifestation of RA, often affecting multiple joints throughout the body. Hence, developing strategies for accurate delivery of therapeutics to inflamed joints is crucial to improving drug delivery efficiency. Herein, we rationally constructed a nanosystem that consists of gold nanoparticles serving as both drug carriers and radiosensitizers, fibroblast activation protein inhibitor (FAPI) as a targeting ligand for pathological neovascularization, and β-cyclodextrin (β-CD) as a host matrix for encapsulating BET inhibitor I-BET151. The targeted delivery enabled selective accumulation of I-BET151 at inflamed joints to mitigate immune activation by inhibiting the abnormal proliferation and migration of synovial fibroblasts in collagen-induced arthritis mice. Single-cell profiling dissected this nanosystem effectively suppressing synovial inflammation by eliminating activated B cells and reversing the hypoxia-inducible factor 1-alpha (Hif 1α)-driven profibrotic and migratory program of fibroblast-like synoviocytes. Combined with low-dose radiotherapy, comprehensive transcriptome standardization and cellular remodeling in RA were achieved. Therefore, our strategy holds considerable promise for advancing the management of rheumatoid arthritis and offers a potent therapeutic modality for refractory RA.

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Cite This Study

Han et al. (2026) studied this question.

synapsesocial.com/papers/69f2f1471e5f7920c6386f32https://doi.org/10.1021/acsnano.6c02626
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