Explores electric double layer dynamics and polarization responsiveness on metal-water interfaces, suggesting a new theoretical framework.
O interfaces exhibit suppressed tunability due to overly loose or dense hydrogen bond structures. Through systematic comparison, we propose a structure-dynamics cooperative balance mechanism, in which interfacial polarization responsiveness is jointly governed by the dynamic fluctuations of water molecules and the spatial continuity of the hydrogen bond network. This framework offers a new theoretical basis for deepening the microscopic understanding of the electric double layer and guiding interfacial modulation.
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Lv et al. (2026) studied this question.
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