The aim is to optimize cascade catalysis using multielement dual-heterostructured catalysts through gradient adsorption engineering.
Established gradient adsorption engineering as a design framework for catalysts.
Compared performance against single-interface and commercial benchmarks.
Demonstrated improved performance of multielement catalysts in cascade reactions.
Outperformed existing single-interface catalysts and commercial benchmarks.
Abstract
, outperforming single-interface and commercial benchmarks. This work establishes gradient adsorption engineering as a general design framework for programming cascade catalysis in multistep reactions.