Uncovers mechanisms enhancing Li+ conduction in solid-state electrolytes, suggesting design principles for improved performance.
= -7.167 eV) compared to hydroxyl groups (-4.457 eV). The cell-TFSI electrolyte forms an in situ LiF-rich solid electrolyte interphase that enables stable lithium plating/stripping cycling for over 1000 h. This work establishes a universal weak solvation and anion immobilization design principle for sustainable, high-performance solid-state polymer electrolytes.
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Yan et al. (2026) studied this question.
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