Experimental and Multiphysics Analysis of Graphene Oxide Paper-Based Ionic Thermoelectric Cell

Approximately 60% of the world’s primary energy is dissipated as waste heat, representing a critical opportunity for energy recovery in sectors such as electro-mobility and fuel cells. Commercial thermoelectric generators (TEGs), predominantly based on bismuth telluride (Bi2Te3), face limitations due to mechanical rigidity, toxicity, and high production costs. This study proposes graphene oxide (GO) as an emerging alternative thanks to its oxygenated functional groups and layered structure as well as GO paper facilitates’ thermal and electrical transport. However, the effective integration of this nanomaterial into solid-state systems under real operating conditions remains a technical challenge. Therefore, this work presents the development, multiphysics modeling, and experimental validation of an innovative TEG cell using GO paper as an active layer. The results demonstrate that the proposed GO-ITC achieves an average of 2.75 times higher generated voltage with a lower thermal gradient as well as an improved equivalent figure of merit (ZT) compared to Bi2Te3-based TEGs. This work contributes to the evaluation of GO-doped materials for voltage generation under specific thermal gradients, providing a lightweight and flexible solution for waste heat harvesting in modern power systems.