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May 6, 2026ChemCatChem

Carbon Nitride With Abundant Nitrogen Vacancies for Methane Oxidation Under Mild Conditions

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Authors

XZX ZhaoHLHongfei LinHYHaibin Yin

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Overview

The study demonstrates enhanced methane oxidation with a nitrogen-vacancy-rich carbon nitride catalyst, suggesting improved oxygenates yield.

Key Points

  • This research aims to explore methane oxidation under mild conditions using a novel catalyst.
  • Utilized nitrogen vacancy-rich graphitic carbon nitride as a catalyst in methane oxidation.
  • Employed H 2 O 2 as the oxidant for the oxidation process.
  • Optimized conditions included 3 MPa CH 4 , 70°C for 1 hour.
  • Achieved an oxygenates yield of 13.42 µmol with the V N -rich CN catalyst.
  • Nitrogen vacancies facilitated H 2 O 2 decomposition into hydroxyl radicals (·OH).
  • Catalytic activity showed a positive correlation with nitrogen vacancy concentration.

Cite This Study

Zhao et al. (2026) studied this question.

synapsesocial.com/papers/69fa983604f884e66b5320a9https://doi.org/10.1002/cctc.70756
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