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Rh-catalyzed C-H allylation and annulation of N-arylpyrazolidinones with MBH adducts | Synapse

May 6, 2026Chemical Communications1 citations

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Rh-catalyzed C-H allylation and annulation of N-arylpyrazolidinones with MBH adducts

KVKshitiz VermaIndian Institute of Technology Guwahati SSSharajit SahaIndian Institute of Technology Guwahati HBHemanga BhattacharyyaIndian Institute of Technology Guwahati

Key Points

This research focuses on developing a Rh-catalyzed annulation method for synthesizing α-pyrazolo[1,2-a]indazole acrylates.
Utilized Rh-catalyzed (4+1)-annulation method
Leveraged MBH adducts as key C1-synthons
Employed air as an oxidant
Involved C-C and C-N bond formation
Successfully synthesized α-pyrazolo[1,2-a]indazole acrylates
Demonstrated C-C bond formation efficiency
Highlighted the role of MBH adducts in synthesis

Abstract

Rh-catalyzed (4+1)-annulation of N-arylpyrazolidinones with MBH adducts has been developed to furnish α-pyrazolo1,2-aindazole acrylates. The use of MBH adduct as C1-synthon, cascade C-C/C-N bond formation, air as the oxidant, substrate...

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Cite This Study

Verma et al. (Thu,) studied this question.

synapsesocial.com/papers/69faa22704f884e66b532c1d https://doi.org/https://doi.org/10.1039/d6cc01732k