What question did this study set out to answer?

The study aims to develop high-performance quasi-solid-state electrolytes for lithium metal batteries.

May 7, 2026Angewandte Chemie

Tailoring Intermolecular Chemistry and Interphases via F, N‐Functionalized Polymer Matrix in High‐Flash‐Point Ether‐Ester Hybrid Electrolytes for Intrinsically Safe Quasi‐Solid‐State Li Metal Batteries

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Authors

HZHuizi ZhangKementerian Pendidikan Malaysia ZNZhiwei NiShandong University YLYuan LiKementerian Pendidikan Malaysia

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Implication

Novel ether-ester hybrid electrolytes enhance ionic conductivity and electrochemical stability in lithium metal batteries, indicating improved performance.

Key Points

The study aims to develop high-performance quasi-solid-state electrolytes for lithium metal batteries.
Developed ether-ester hybrid electrolytes using in situ copolymerization of TFEA and IEM.
Investigated the effects of functionalized polymer matrix on Li+ solvation structure and interphase formation.
Measured ionic conductivity and electrochemical performance of Li||LiFePO4 and Li||NCM811 cells.
Achieved a high room-temperature ionic conductivity of 2.2 × 10−3 S cm−1.
Demonstrated 93% capacity retention over 1,000 cycles in Li||LiFePO4 cells.
Showed 80% capacity retention over 300 cycles in Li||NCM811 cells, achieving specific energy of 302.64 Wh kg−1.

Cite This Study

Zhang et al. (2026) studied this question.

synapsesocial.com/papers/69fbef68164b5133a91a34b2 https://doi.org/10.1002/ange.1984422

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Implication

Novel ether-ester hybrid electrolytes enhance ionic conductivity and electrochemical stability in lithium metal batteries, indicating improved performance.

Tailoring Intermolecular Chemistry and Interphases via F, N‐Functionalized Polymer Matrix in High‐Flash‐Point Ether‐Ester Hybrid Electrolytes for Intrinsically Safe Quasi‐Solid‐State Li Metal Batteries

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Key Points

Cite This Study

Tailoring Intermolecular Chemistry and Interphases via F, N‐Functionalized Polymer Matrix in High‐Flash‐Point Ether‐Ester Hybrid Electrolytes for Intrinsically Safe Quasi‐Solid‐State Li Metal Batteries

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