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May 10, 2026Crystals0 citationsOpen Access

The Synthesis, Spectroscopic and Structural Study of a Copper(II) Complex with a (3-py)2Hg Linker: A Zig-Zag Chain Paddle-Wheel Coordination Polymer

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APAlexandra PopBabeș-Bolyai UniversityCSCristian SilvestruBabeș-Bolyai UniversityLPLucian Cristian PopBabeș-Bolyai University

Key Points

  • The aim is to synthesize and characterize a copper(II) complex using a (3-py)2Hg linker.
  • Reaction of (3-py)2Hg with Cu(OAc)2·H2O in a 1:2 molar ratio to synthesize the polymer.
  • Characterization via elemental analysis, IR, UV-Vis spectroscopies, thermogravimetric analysis, and powder X-ray diffraction.
  • Structural determination using single-crystal X-ray diffraction.
  • The new polymer [(3-py)2Hg{Cu2(OAc)4}] exhibits a zig-zag 1D chain structure.
  • Characterization reveals a strong bimetallic interaction with structural support from interchain interactions.
  • The UV-Vis properties of solid (3-py)2Hg were also detailed for comparison.

Abstract

The reaction of (3-py) 2Hg (1) with Cu (OAc) 2·H2O, in a 1: 2 molar ratio, afforded the isolation of (3-py) 2HgCu2 (OAc) 4n (2). This new bimetallic coordination polymer based on copper (II) - and mercury (II) -containing building blocks was characterized by an elemental analysis, IR and UV-Vis spectroscopies, a thermogravimetric analysis, and powder X-ray diffraction. For comparison, the UV-Vis properties of solid 1 are also reported. The structure of both 1 and 2 were established by single-crystal X-ray diffraction. The structural analysis of 2 shows a zig-zag 1D chain with alternating (3-py) 2Hg molecules and Cu2 (OAc) 4 fragments connected via N → Cu coordinative bonds. Further interchain Hg···O, H···π, and π···π interactions support a 2D layer of zig-zag chains.

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Cite This Study

Pop et al. (2026) studied this question.

synapsesocial.com/papers/6a002162c8f74e3340f9c386https://doi.org/10.3390/cryst16050314
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