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electroreduction on copper. The results demonstrate how DRS can uncover solvent dynamics, charging delays, and memory effects that elude current-only, single frequency, or modality analyses. Rather than imposing predefined mechanistic assumptions, DRS allows the system's natural dynamical structure to emerge. We discuss the conceptual implications and practical considerations for implementing DRS across catalytic systems. By acknowledging time-domain complexity, DRS offers an alternative axis of mechanistic insight into the emergent behaviors that govern catalytic activity, selectivity, and stability.
Sinausia et al. (Fri,) studied this question.