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A newly designed millimeter-wave spectrometer has been employed for precise measurements of the millimeter-wave rotational spectrum of HCNO. Absorptions in several excited vibrational states as well as the ground state could be measured. The present paper presents the observed frequen cies and molecular constants obtained for the ground state and the first excited state of v 4 and of v 5 , the vibrational bending modes
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Winnewisser et al. (1971) studied this question.
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