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DFT study demonstrates efficient hydrogenation of Al(I) monomers using low-valent Group 13 complexes, indicating effective catalysis.
addition, leading to lower activation barriers relative to N,N-amidinate-supported systems. Furthermore, our calculations validate that amidophosphine-stabilized In(I) carbenoid can efficiently catalyze the hydrogenation of both N,P- and N,N-chelated Al(I) monomers to yield the corresponding Al(III) dihydrides.
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Li et al. (2026) studied this question.
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