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Herein we report a one‐pot protocol for the deracemisation of chiral benzylic amines employing a novel monoamine oxidase–ω‐transaminase cascade, allowing access to enantiopure compounds in >99 % ee . We also demonstrate that the same enzymatic cascade can be employed for the dealkylation of secondary amines with >99 % conversion.
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O’Reilly et al. (2014) studied this question.
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