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A quantum time-dependent wave-packet method is used to investigate the predissociation dynamics of a model system (IBr). The dissociation is characterized by a two-state model. The effect of nonadiabatic coupling on the absorption and continuum Raman spectra is examined. The dissociation dynamics and nonadiabatic transitions are also studied in the time domain using femtosecond pulses.
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Hua Guo (1993) studied this question.
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