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/K)] provides superior catalytic performance, reducing the oxygen evolution overpotential by ∼200-400 mV. Density functional theory simulations provide an illustration of the electronic properties (density of states and localization of orbitals) that promote catalysis in the layer-segregated materials over those of homogeneous composition. This study reveals that atomic preorganization of metal ions within layered catalysts plays a more crucial role than the overall metal composition in enhancing catalytic efficiency for oxygen evolution.
Ding et al. (Mon,) studied this question.
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