Demonstrates a bulk reversible non-stoichiometric reaction in a lithium amide/imide system, suggesting implications for hydrogen storage technologies.
We demonstrate, through structural refinement from synchrotron X-ray diffraction data, that the mechanism of the transformation between lithium amide and lithium imide during hydrogen cycling in the important Li-N-H hydrogen storage system is a bulk reversible reaction that occurs in a non-stoichiometric manner within the cubic anti-fluorite-like Li-N-H structure.
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David et al. (2007) studied this question.
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