Explores how solvent coordination affects single-molecule magnet performance, suggesting significant improvement potential.
however, the other two complexes are single-molecule magnets (SMM). Obviously, the progressive replacement of the coordinated solvent molecules of methanol by DMF systematically slows down the magnetic relaxation and improves the SMM performance. This is a typical example of using two types of coordination solvent molecules to tune SMM performance, providing some hints for enhancing cluster-based SMM performance. Theoretical calculations further elucidated the solvent-mediated SMM tuning effect by exploring the magneto-structural correlation.
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Deng et al. (2026) studied this question.
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