Crystals of Bound States in the Magnetization Plateaus of the Shastry-Sutherland Model

Using infinite projected entangled-pair states, we show that the Shastry-Sutherland model in an external magnetic field has low-magnetization plateaus which, in contrast to previous predictions, correspond to crystals of bound states of triplets, and not to crystals of triplets. The first sizable plateaus appear at magnetization 1/8, 2/15 and 1/6, in agreement with experiments on the orthogonal-dimer antiferromagnet SrCu2(BO3)2, and they can be naturally understood as regular patterns of bound states, including the intriguing 2/15 one. We also show that, even in a confined geometry, two triplets bind into a localized bound state with Sz=2. Finally, we discuss the role of competing domain-wall and supersolid phases, as well as that of additional anisotropic interactions.