The eruption of the Eyjafjallajökull volcano, Iceland, in April and May 2010 caused unprecedented disruptions of European air traffic showing that timely monitoring of volcanic ash and SO 2 dispersion as well as the corresponding plume heights are important for aviation safety. This paper describes the observations of SO 2 and BrO columns in the eruption plume and the determination of the SO 2 plume height using the GOME‐2 satellite instrument. During the eruptive period in May 2010, SO 2 total columns of up to ∼20 DU and BrO columns of ∼7.7 × 10 13 molec/cm 2 were detected. The BrO/SO 2 ratio estimated from the GOME‐2 observations of the Eyjafjallajökull eruption varies from 1.1 × 10 −4 to 2.1 × 10 −4 . The SO 2 plume heights estimated from the GOME‐2 observations on 5 May range from 8–13 km and mostly agree within 1–3 km with visual observations, radar data and modeling results. Furthermore, the GOME‐2 SO 2 observations are compared with in situ measurements of the DLR Falcon aircraft on 17 and 18 May 2010 and with Brewer instruments at Valentia, Ireland and Hohenpeissenberg, Germany. The SO 2 columns derived from the Falcon profile measurements range from 0.6–4.7 DU and the comparison with the GOME‐2 measurements shows a good agreement, mainly within 1 DU. The Brewer observations at Hohenpeissenberg also agree well with the GOME‐2 measurements with a daily average SO 2 column of ∼1.3 DU during the overpass of the SO 2 cloud on 18 May, whereas the Brewer instrument at Valentia shows up to 50% higher SO 2 columns (∼8 DU) on 11 May.
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