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A visible light-mediated C(sp3)–H amination strategy enabled by ligand-to-metal charge transfer and iron catalysis allows for efficient C(sp3)–N bond construction under mild conditions with broad functional group tolerance. Novelty: ClaimNovelty.METHODOLOGICAL. Consensus alignment: ConsensusAlignment.NEUTRAL.

Iron-Catalyzed C(sp 3 )–H Amination Enabled by Visible-Light β-Homolysis

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