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Experimental and computational approaches reveal the mechanism for synthesizing eight-membered carbocyclic rings.
An access to functionalised eight‐membered carbocyclic ring compounds was developed by simply stirring an unusual vinylogous Donor‐Acceptor Cyclopropane (DAC) in boiling o ‐xylene. Both experimental and computational studies were performed to explain the diastereoselectivity/regioselectivity transfer observed and to provide an overall picture of the mechanism. magnified image
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Masson et al. (2023) studied this question.
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