Regulating the twist: Tunable supramolecular chirality is induced in an achiral helical self-assembly (P, M; see picture) by hydrogen-bonded chiral guest molecules (yellow and purple rods). Chiroptical probing of the π-conjugated chromophore reveals the mechanistic pathways of chiral induction. “Majority rules” and “sergeant and soldiers” experiments give insight into the chiral amplification in the stacks.
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George et al. (2007) studied this question.
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