The rate-determining step for ammonia synthesis over Ru catalysts supported by electrides, such as [Ca ₂₄ Al ₂₈ O ₆₄ ] ⁴⁺ (e ⁻ ) ₄ and Ca ₂ N:e ⁻ , is suggested to be the surface reactions of N and H adatoms, in which case the Langmuir–Hinshelwood model should be used to describe the kinetics.
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Kobayashi et al. (2016) studied this question.
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