A theory for covalent octahedrally co-ordinated Yb 3+ is developed. A system of molecular orbitals is set up, and the orbital contribution to the g value and the hyperfine interactions with the ligand nuclei are evaluated for the lowest doublet. The model neglects electron transfer into central ion 5d, 6s and 6p orbitals.
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J. H. M. Thornley (1966) studied this question.
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