Diacetylene macromonomers functionalized with a β-sheet-forming oligopeptide and a hydrogenated poly(isoprene) coil segment self-assembled into supramolecular polymers with a double-helical, tubular topology and a diameter of a few nanometers. Subsequent “1D topochemical polymerization” affords poly(diacetylene)s with a conjugated backbone and a high degree of biochemically relevant functionalization, as well as a defined hierarchical structure.
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Jahnke et al. (2006) studied this question.
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