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Self-phase modulation has been observed for ultrashort pulses of wavelength 800nm propagating through a 1 cm-long Ta2O5 rib waveguide. The associated nonlinear refractive index n2 was estimated to be 7.23x10-19 m2/W, which is higher than silica glass by more than one order of magnitude. Femtosecond time of flight measurements based on a Kerr shutter configuration show that the group velocity dispersion is small at a wavelength of 800 nm, confirming that dispersion may be neglected in the estimation of n2 so that a simplified theory can be used with good accuracy.
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Tai et al. (2004) studied this question.
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