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We have used subpicosecond laser pulses to launch ultrahigh strain rate (∼109s−1) nonlinear acoustic waves into a 4:1 methanol-ethanol pressure medium which has been precompressed in a standard diamond anvil cell. Using ultrafast interferometry, we have characterized acoustic wave propagation into the pressure medium at static compression of up to 24GPa. We find that the velocity is dependent on the incident laser fluence, demonstrating a nonlinear acoustic response which may result in a shock wave behavior. We compare our results to low strain rate acoustic data. This technique provides controlled access to regions of thermodynamic phase space that is otherwise difficult to obtain.
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Armstrong et al. (2008) studied this question.
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