It is shown that the methods proposed by Montroll and Kroll for deriving the lattice frequency spectrum from the experimental specific heat curve will in practice yield only a `smoothed' spectrum, averaged over a range of 1.6: 1 or more in frequency. Any practicable improvement in experimental accuracy will reduce this smoothing only slightly. The same smoothed spectrum can be derived more simply by a procedure involving only one quadrature, and a still simpler trial-and-error method is also described and illustrated.
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Robert G. Chambers (1961) studied this question.
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