Conductive and flexible multi‐walled carbon nanotube/polydimethylsiloxane composites made with naphthalene/toluene mixture

Conventional conductive materials face challenges when utilizing them for flexible and wearable electronics and soft robotics. Carbon nanotube/polydimethylsiloxane (CNT/PDMS) composites are a promising alternative to the conventional hard conductors because they are light and can realize large deformation. To date, well dispersion of CNTs into PDMS to increase conductivity while maintaining flexibility remains challenging. We aimed at developing highly electrically conductive and flexible multi‐walled carbon nanotube/PDMS (MWCNT/PDMS) composites. To this end, we proposed a method to enhance the dispersion of MWCNTs into PDMS using naphthalene and toluene. Our results showed that the addition of naphthalene and toluene into the composites improved dispersion of the MWCNTs and increased the direct current (DC) electrical conductivity. We also found that the morphology of primary aggregates of the MWCNTs influenced the DC electrical conductivity of the composites.