A three−dimensional semiclassical model for vibrational/rotational transitions has been extended to include an infinite order treatment of the rotational transitions. An analytical expression for the transition probabilities is obtained by using an effective potential and a simple collision trajectory. Numerical results for the Ar−N2 and the I2(B3Π0u+) + He4 systems have been obtained.
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Gert D. Billing (1975) studied this question.
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