We report results of a molecular-beam magnetic-resonance study of the paramagnetic Van der Waals molecule KAr. The experiment yields a value for the spin-rotation interaction γ→S·→N, where →S and →N are, respectively, the electronic and rotational angular momentum. The average spin-rotation constant in KAr is γ=0.24(1) MHz.
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Mattison et al. (1974) studied this question.
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