Sulfur dioxide clusters prepared in seeded, pulsed, supersonic molecular beams have been scattered from single crystal surfaces under ultrahigh vacuum conditions with the aim to investigate chemical changes (e.g. fragmentation) and cluster‐surface interaction with regard to certain experimentally accessible conditions (cluster size, kinetic energy, type and temperature of the surface). First measurements are reported which show that (SO 2 ) n ( n > 3) dissociation may occur yielding both, positively and negatively charged ionization products. Possible cluster‐surface interaction mechanisms are discussed.
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Christen et al. (1992) studied this question.
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