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The structure of a liquid can be investigated through the photostatistics of scattered light. A theoretical approach is given in which the deviation from the Poisson distribution, followed by the photons of a single-mode laser beam, is connected with the two- and four-particle distribution functions of the scattering medium. In particular, the presence of the Mandelstam-Brillouin doublet is put into evidence through the time behavior of a non-Poissonian statistical term, by using an explicit form of the two-particle correlation function.
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Bertolotti et al. (1967) studied this question.
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