Design and operation of a new apparatus for electron–ion coincidence studies is described. For ionic fragmentation of inner-shell excited molecules, the degree of decomposition of the molecule depends on where valence two holes are created by a subsequent Auger decay. Auger electron–photoion coincidence (AEPICO) measurements are indispensable for studying the ionic fragmentations of the core-excited molecules, because these measurements can define the fragmentation products produced from a certain Auger final state. Experimental results for SiF4 are demonstrated as an example for the performance of the apparatus.
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Shigemasa et al. (1992) studied this question.
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