Two polymorphs of KCsWP ₂ O ₉ exhibit a large SHG response due to non-bonding O-2p orbitals and strong orbital interactions of W-5d orbitals and O-2p orbitals, the orientations of the dipole moments of WO ₆ are also beneficial for the large SHG response.
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Baiheti et al. (2020) studied this question.
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